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CHAPTER 12






                                        Ultrafast Solid-State


                                                                   Lasers






                      Sterling Backus
                      Vice President, Research and Development, Kapteyn-Murnane
                        Laboratories, Inc., Boulder, Colorado





                 12.1  Introduction
                      Over the past 15 years, ultrafast laser technology and its applications
                      have  progressed  by  leaps  and  bounds,  ever  since  the  widespread
                      introduction of solid-state ultrafast laser materials in the early 1990s.
                                                                               1
                      In  1990,  the  state-of-the-art  femtosecond  (fs)  laser  used  dye  laser
                      media  and  could  generate  output  powers  in  the  tens  of  milliwatt
                      (mW) range, with pulse durations of ~100 fs. The successful applica-
                      tion  of  titanium-doped  sapphire  (Ti:sapphire)  to  ultrafast  lasers
                      immediately resulted in an order of magnitude increase in average
                      power (to ~1 W), as well as in the ability to easily and reliably gener-
                                             2
                      ate pulses of less than 10 fs.  This technological advance has since led
                      to a tremendous broadening of the field of ultrafast science, and more
                      applications could be successfully implemented with the new gener-
                      ation of lasers. For example, the use of ultrafast lasers for machining
                      and materials ablation began in the mid-1980s, with the realization
                      that the high-intensity laser–matter interaction is fundamentally dif-
                      ferent on femtosecond (compared with picosecond or nanosecond)
                      timescales,  allowing  for  a  much  more  precise  and  well-controlled
                             3
                      ablation.  Peak powers into the petawatt (PW) regime have been real-
                                                 4–6
                      ized,  owing  to  ultrafast  pulses.   This  high-peak-power  capability
                      has also defined many other applications throughout physics, chem-
                      istry, and biology. However, the “real world” applications of femto-
                      second  lasers  only  became  practical  with  the  development  of
                      high-power solid-state (predominantly Ti:sapphire) lasers. Femtosec-
                      ond lasers are now used in a few industrial and medical settings, such

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