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Unstable Nuclei and Radioactive Decay              61


                (e)  The  total angular momentum PI of the system must be conserved,  i.e.

                                      (PI)1  +  (1191)2 --" (/91)3 +  (PI)4         (4.8)

                Since there exist two types of angular momentum, one caused by orbital movement of the
               individual nucleons and the other due to the intrinsic spin of the nucleons (internal angular
               momentum),  a  more practical  formulation of (4.8)  is

                                         AI=I  3  +14-I1-I   2                      (4.9)

               where  I  is the  (total)  nuclear spin quantum  number.  The quantum rule  is

                                           AI  =  0,  1,  2,  3,  ...              (4.10)

               i.e.  the change of nuclear  spin in a reaction  must have an  integral  value.
                The  three  first  laws  are  general  in  classical  physics;  the  last  two  refer  particularly  to
               nuclear  reactions.  In  Ch.  10  and  1 1  other  conservation  laws  are  discussed  for  nuclear
               reactions,  but  these are  less  important  in radioactive decay.


                                            4.3.  Alpha  decay


               4.3.1.  Detection

                Alpha particles  cause  extensive ionization in  matter.  If the particles  are  allowed to pass
               into a gas,  the electrons  released by the ionization can be collected on a positive electrode
               to  produce  a  pulse  or  current.  Ionization  chambers  and  proportional  counters  are
               instruments  of this  kind,  which  permit  the  individual  counting  of each  t~-particle emitted
               by a  sample.  Alpha  particles  interacting with  matter may also cause molecular excitation,
               which can  result  in fluorescence.  This  fluorescence  -  or scintillation  -  allowed the  first
               observation of individual nuclear particles.  The ionization in semiconductors caused by t~-
               particles  is now  the most common means of detection,  see Ch.  8.


               4.3.2.  Decay energy

                Alpha  decay  is observed for the elements heavier than  lead and  for a  few nuclei  as light
               as  the  lanthanide  elements.  It can be written  symbolically as

                                           ~X --, z_2XA-4 +  ~He                   (4.11)

                We  use  X  to  indicate  any  element  defined  by  its  nuclear  charge,  Z  and  Z-2  in  this
               equation.  Examples  are  given  in  Ch.  1,  and  can  be  found  e.g.  in  the natural  radioactive
               decay  series,  see next  chapter.
                The decay energy can be calculated  from the known atomic  masses,  because the binding
              energy  released  (spontaneous  decay  processes  must  be  exoergic)  corresponds  to  a
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