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4  CO,  isotope lasers and Their Applicaticns   137

                      To  assess  the  frequency  differences  between  the  results  published  by
                   Bradley  er  al.  [37] and those  to be published by  Maki  et al. [38]. I compiled
                   Tab'le 11. which  shows  the  frequency  differences  in kilohertz  for  the  regular
                   band  lasing  transitions  (differing  by  A/  = 8  or  10) in  the  four  CO,  isotopic
                   species  to  be  published  by  Maki  er  a]. [38]. Similar to  the  case  in-Tables  2
                   through  IO, the  horizontal lines  in Table  11 demarcate  the  boundaries  in each
                   vibrational-rotational  branch beyond which higher J  lines were not measured in
                   the Bradley et al. database.
                      Table  11 clearly  indicates that  within  the  database  given in Bradley  er  al.
                   only one transition.  the II-R(50) of  12C1807, differs by  more than  11 kHz.  For
                   most other transitions within the measured database in [37] the frequency differ-
                   ences are only a few kilohertz and would be even less had we taken into account
                   the -2.9-kHz  correction to be applied to the I-R(30) WlSO,  absolute frequency
                   reference used in Bradley et al. [37].
                       At  this  stage of  development it  appears  that  even more  refined techniques
                   will be necessary to attain another order of magnitude improvement in the preci-
                   sion and accuracy of CO, beat frequency measurements than was obtained with
                   the relatively simple two-channel heterodyne system depicted in Fig. 13. Such an
                   improved  system  was  developed at MIT Lincoln Laboratory  in order to obtain
                   reliable measurements of pressure shifts in the CO,  laser system [76.111.112]. A
                   brief outline  of  the  improved heterodyne  setup and the results of pressure shift
                   measurements is given in the next section. However, before leaving the subject of
                   absolute frequency calibration of CO, laser transitions, I would like to repeat here
                   the dedication written for the paper b;  Bradley et al. [37]:
                        The  authors  nould  like  to  dedicate  this  Lvork  to  th2  memory  of  the  late  Russell
                      Petersen, who did so much for the measurement  of absolute frequencies  at optical wave-
                       lengths. and uhos2 work has been an essential foundation stone for this paper. Russ was
                       also a true friend, and his premature  death leaves a large gap in the lives of psople who
                       were privileged to ho~v him.
                   I was gratified to see a very similar dedication to F. R. Petersen in the forthcom-
                   ing paper by Maki et al. [38].


                   7 0.  PRESSURE SHIFTS IN LINE-CENTER-STABILIZED CO, LASERS

                       In  the  very  first  publication  on  the  standing-wave  saturation  resonances
                   observed in the 4.3-pm fluorescence band of  CO,,  Freed and Javan drew atten-
                   tion  to  the  phenomenon  (see Fig.  1 in  [48]) that  the  center  frequency  of  the
                   standing-wave  saturation resonance shifted by about 0.33 MHz on the low-fre-
                   quency side of the peak in the broad background curve. (Note that in the actual
                   Appl. Phys  Lett. publication  exactly  the reverse  direction  was  statcd and indi-
                   cated by the arrou s. This error was caught shortly after publication and a correc-
                   tion erratum was included with reprints.) The two-mirror laser (shown in Fig. 9)
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