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CHAPTER 18 • Causes of Warming over the Last 125 Years  333


                     N

                    60°


                    30°


                     0°


                    30°

                                                               3
                                                    Sulfate (mg/m )  2–6    6–10    >10
                    60°
                     S           120°        60°          0°          60°         120°
                       W                                                                      E
        FIGURE 18-10 Sulfate aerosol plumes Sulfur dioxide emissions from industrial smokestacks in
        the North American Midwest, Eastern Europe, and China produce sulfate aerosols that prevailing
        winds carry eastward in large plumes. (Adapted from R. J. Charlson et al., “Perturbation of the
        Northern Hemisphere Radiative Balance by Backscattering from Aerosols,” Tellus 43 [1991]: 152–63.)


           Part of the history of SO emissions is recorded in
                                 2
        Greenland ice (Figure 18–11). Throughout the 1800s,
        industrial SO emissions had been smaller than those
                    2
        from natural sources, but by the middle 1900s, industry      Volcanic
        emissions became the dominant SO source. The sul-            explosions
                                       2                       Sulfate concentration
        fate concentration in Greenland ice rose sharply during
        World War II industrialization. Concentrations in
        Greenland ice began to drop sharply after 1980, when
        the United States (and then other nations) acted to limit
                                                                 0
        SO emissions.                                                 1700       1800       1900       2000
           2
           Climate scientists have inferred that the large plumes  A  Sulfate concentration in ice cores
        of sulfate aerosols cause regional cooling downwind from  100
        smokestack sources. Like sulfate aerosols created by vol-
        canic explosions, industrial sulfate particles reflect and
        scatter some of the incoming solar radiation back to
        space and keep it from reaching Earth’s surface. The
        reduction in radiation cools climate regionally, and these  SO 2  (gigatons/year)  50  Human
        effects show up in tabulations of global mean tempera-                             emissions
        ture change.
           A second potential climatic effect of sulfate aerosols    Range of natural emissions
        is less well understood. The tiny particles form natural
        centers (nuclei) around which water vapor can condense,  0
        forming droplets and then clouds. Clouds can have two         1700       1800       1900       2000
                                                                                    Year
        opposing effects on climate: the surfaces of thick clouds
                                                            B  Estimated global SO  emissions
        can reflect more incoming solar radiation and cool                     2
        climate, but thinner, higher clouds can also absorb more  FIGURE 18-11 Preindustrial and anthropogenic sulfates
        outgoing radiation from Earth’s surface and increase the  (A) Measured sulfate concentrations in Greenland ice
        greenhouse effect. Because sulfate aerosols mainly affect  reveal a significant regional increase since the nineteenth
        low-level clouds, their indirect effects are thought to  century. (B) Estimated global SO emissions from
                                                                                     2
        cool climate, but the amount is highly uncertain.   smokestacks now exceed natural emissions. (A: Adapted from
                                                            P. A. Mayewski et al., “An Ice-Core Record of Atmospheric
          IN SUMMARY, the net global effect of increased    Responses to Anthropogenic Sulphate and Nitrate,” Atmospheric
          sulfate aerosols is thought to be a cooling, but   Environment 27 [1990]: 2915–19. B: Adapted from R. J. Charlson
          estimates of the size of the cooling vary widely.  et al., “Climate Forcing by Anthropogenic Aerosols,” Science 255
                                                            [1992]: 423–30.)
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